Bis(μ-2-tert-butyl­phenyl­imido-1:2κ2 N:N)chlorido-2κCl-(diethyl ether-1κO)(2η5-penta­methyl­cyclo­penta­dien­yl)lithiumtantalum(V)

نویسندگان

  • Jacqueline M. Cole
  • Michael C. W. Chan
  • Vernon C. Gibson
  • Judith A. K. Howard
چکیده

In the title compound, [LiTa(C(10)H(15))(C(10)H(13)N)(2)Cl(C(4)H(10)O)], the Ta(V) atom is coordinated by a η(5)-penta-methyl-cyclo-penta-dienyl (Cp*) ligand, a chloride ion and two N-bonded 2-tert-butyl-phenyl-imide dianions. With respect to the two N atoms, the chloride ion and the centroid of the Cp* ring, the tantalum coordination geometry is approximately tetra-hedral. The lithium cation is bonded to both the 2-tert-butyl-phenyl-imide dianions and also a diethyl ether mol-ecule, in an approximate trigonal planar arrangement. The Ta⋯Li separation is 2.681 (15) Å. In the crystal, a weak C-H⋯Cl inter-action links the mol-ecules. When compared to the 2,6-diisopropyl-phenyl-imide analogue ('the Wigley derivative') of the title compound, the two structures are conformationally matched with an overall r.m.s. difference of 0.461Å.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Bis[μ-N,N′-bis(2,6-diisopropylphenyl)ethene-1,2-diamido]-1,4(η2);1:2κ4 N:N;3:4κ4 N:N-bis(diethyl ether)-1κO,4κO-di-μ-hydrido-2:3κ4 H:H-2,3-dichromium(II)-1,4-dilithium(I) pentane hemisolvate

The title compound, [Cr(2)Li(2)(C(26)H(36)N(2))(2)(μ-H)(2)(C(4)H(10)O)(2)]·0.5C(5)H(12), is a binuclear chromium complex bridged by two hydrogen atoms. Each chromium atom is coordinated in a distorted square-planar geometry by one chelating bis-(2,6-diisopropyl-phen-yl)ethene-1,2-diamido ligand via its two N atoms. Additionally, two diametrically opposed lithium ether adducts coordinate in an η...

متن کامل

Crystal structure of μ-1κC:2(η2)-carbonyl-carbonyl-1κC-chlorido-2κCl-μ-chlorido­borylene-1:2κ2 B:B-[1(η5)-penta­methyl­cyclo­penta­dien­yl](tri­cyclo­hexyl­phosphane-2κP)iron(II)platinum(II) benzene monosolvate

In the mol-ecular structure of the dinuclear title compound [η(5)-(C5(CH3)5)(CO)Fe{(μ-BCl)(μ-CO)}PtCl(P(C6H11)3)]·C6H6, the two metal atoms, iron(II) and platinum(II), are bridged by one carbonyl (μ-CO) and one chlorido-borylene ligand (μ-BCl). The Pt(II) atom is additionally bound to a chloride ligand situated trans to the bridging borylene, and a tri-cyclo-hexyl-phosphane ligand (PCy3) trans ...

متن کامل

Bis(methanol-1κO)tetra-μ-pyridazine-1:2κ4 N:N′;2:3κ4 N:N′-di-μ-thio­cyanato-1:2κ2 N:N;2:3κ2 N:N-tetrathio­cyanato-1κ2 N,3κ2 N-trinickel(II) methanol tetra­solvate

Reaction of an excess nickel(II) thio-cyanate with pyridazine leads to single crystals of the title compound, [Ni(3)(NCS)(6)(N(2)C(4)H(4))(4)(CH(3)OH)(2)]·4CH(3)OH. The crystal structure consists of trimeric discrete complexes, in which two Ni(II) cations are coordinated by two terminal and one μ-1,1 bridging thio-cyanato anions, one methanol mol-ecule and two bridging pyridazine ligands, where...

متن کامل

[N,N′-Bis(2,6-diisopropyl­phen­yl)pentane-2,4-diamine­(1–)-2κ2 N,N′]-μ2-chlorido-1:2κ2 Cl:Cl-chlorido-2κCl-bis­(1,2-di­methoxy­ethane-1κ2 O,O′)iron(II)lithium

In the title compound, [FeLi(C(29)H(41)N(2))Cl(2)(C(4)H(10)O(2))(2)], the Fe(II) atom is coordinated by two N and two Cl atoms, generating a distorted FeN(2)Cl(2) tetra-hedral geometry. Additionally, one of the chloride atoms bridges to a lithium ion, which is solvated by two dimethoxy-ethane mol-ecules and is coordinated in a distorted trigonal-bipyramidal environment. The central Fe, Cl (× 2)...

متن کامل

Crystal structure of a mixed-ligand dinuclear Ba—Zn complex with 2-meth­oxy­ethanol having tri­phenyl­acetate and chloride bridges

The dinuclear barium-zinc complex, μ-chlorido-1:2κ(2) Cl:Cl-chlorido-2κCl-bis-(2-meth-oxy-ethanol-1κO)bis-(2-meth-oxy-ethanol-1κ(2) O,O')bis-(μ-tri-phenyl-acetato-1:2κ(2) O:O')bariumzinc, [BaZn(C20H15O2)2Cl2(C3H8O2)4], has been synthesized by the reaction of barium tri-phenyl-acetate, anhydrous zinc chloride and 2-meth-oxy-ethanol in the presence of toluene. The barium and zinc metal cations in...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:

دوره 67  شماره 

صفحات  -

تاریخ انتشار 2011